Microphysical process rates and global aerosol-cloud interactions

The relative importance of different microphysical processes in a climate model is analyzed, and the autoconversion and accretion processes are found to be critical to the condensate budget in most regions. A simple steady-state model of warm rain formation is used to illustrate that the diagnostic rain formulations typical of climate models may result in excessive contributions from autoconversion, compared to observations and large eddy simulation models with explicit bin-resolved microphysics and rain formation processes.

The behavior does not appear to be caused by the bulk process rate formulations themselves, because the steady-state model with the same bulk accretion and autoconversion has reduced contributions from autoconversion. Sensitivity tests are conducted to analyze how perturbations to the precipitation microphysics for stratiform clouds impact process rates, precipitation susceptibility and aerosol-cloud interactions (ACI).