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Table · dataset · 2026

High-Damping Elastomers Enabled by Precise Regulation of Polyborosiloxane Relaxation Behaviors

Listed in ZivaHub and Deakin Research Online — shown once because both records carry DOI 10.1021/acs.chemmater.6c02055.s001

Viscoelastic polymer materials exhibiting high damping capacity within a specified frequency–temperature range effectively dissipate mechanical energy as heat, thereby mitigating damage induced by vibrations and impact loads.

Description

However, developing a convenient method for precisely designing damping materials with tunable energy dissipation properties across a desired frequency–temperature range remains challenging. Herein, we present a strategy for fabricating high-damping polyborosiloxane (PBS) elastomers (PBSEs) with tunable damping performance across a specified frequency–temperature range.

This is achieved by precisely modulating the PBS relaxation behaviorspecifically, through systematic variation of both the B–O bond content and the molecular weight of the PDMS diol precursors. We found that the resultant PBSEs exhibit controllable high-damping performance across an ultrawide frequency range (tan <i>δ</i> > 0.3, 10<sup>–3</sup> to 10<sup>2</sup> Hz) and temperature range (tan <i>δ</i> = 0.5–0.6, −20 to 150 °C).

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Moreover, PBSEs exhibit excellent impact-protective performance compared with commercial materials and attenuate impact force by more than 95%. This unique design concept will provide a convenient approach to developing advanced damping materials.

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ZivaHuboai:figshare.com:article/3403047610 d agoJSON v1
Deakin Research Onlineoai:figshare.com:article/3403047610 d agoJSON v1
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