Effect of wind speed on the size distribution of gel particles in the sea surface microlayer: Insights from a wind wave channel experiment

Wind speeds > 8 m s−1 decreased the slope of CSPSML size distribution significantly in the absence of autotrophic growth. For the slopes of TEP and CSP size distribution in the bulk water, no significant difference was observed between high and low wind speeds. Changes in spectral slopes between high and low wind speed were higher for TEPSML than for CSPSML, indicating that the impact of wind speed on size distribution of gel particles in the SML may be more pronounced for TEP than for CSP, and that CSPSML are less prone to aggregation during the low wind speeds.

Addition of an E. huxleyi culture resulted in a higher contribution of submicron gels (0.4–1 µm) in the SML at higher wind speed (> 6 m s−1), indicating that phytoplankton growth may potentially support the emission of submicron gels with sea spray aerosol.