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Data · dataset · 2026

Characteristics and sources of carbonaceous aerosols from Shanghai, China

Listed in National Center for Atmospheric Research

An intensive investigation of carbonaceous PM2.5 and TSP (total suspended particles) from Pudong (China) was conducted as part of the MIRAGE-Shanghai (Megacities Impact on Regional and Global Environment) experiment in 2009.

Description

Data for organic and elemental carbon (OC and EC), organic species, including C17 to C40 n-alkanes and 17 polycyclic aromatic hydrocarbons (PAHs), and stable carbon isotopes OC (σ¹³COC) and EC (σ¹³CEC) were used to evaluate the aerosols' temporal variations and identify presumptive sources.

High OC/EC ratios indicated a large fraction of secondary organic aerosol (SOA); high char/soot ratios indicated stronger contributions to EC from motor vehicles and coal combustion than biomass burning. Diagnostic ratios of PAHs indicated that much of the SOA was produced via coal combustion. Isotope abundances (σ¹³COC = -24.5 ± 0.8% and σ¹³CEC = -25.1 ± 0.6%) indicated that fossil fuels were the most important source for carbonaceous PM2.5 (particulate matter less than 2.5 micrometers in diameter), with lesser impacts from biomass burning and natural sources.

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An EC tracer system and isotope mass balance calculations showed that the relative contributions to total carbon from coal combustion, motor vehicle exhaust, and SOA were 41%, 21%, and 31%; other primary sources such as marine, soil and biogenic emissions contributed 7%. Combined analyses of OC and EC, n-alkanes and PAHs, and stable carbon isotopes provide a new way to apportion the sources of carbonaceous particles.

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Provenance · 1 source records, 7 field assertions
SourceKeyLast seenRaw
National Center for Atmospheric Researchf4888275-c0d6-4a78-be75-d395dc9ad7a211 d agoJSON v1
FieldAssertionExtractorEvidence
concepts[field].local:field:earth-environmentalmapping · data ucar educonnector:data_ucar_edu@1.0.0
concepts[field].local:field:ocean-atmosphericmapping · data ucar educonnector:data_ucar_edu@1.0.0
created_datesource · data ucar educonnector:data_ucar_edu@1.0.0
descriptionsource · data ucar educonnector:data_ucar_edu@1.0.0/notes
publication_datesource · data ucar educonnector:data_ucar_edu@1.0.0
titlesource · data ucar educonnector:data_ucar_edu@1.0.0/title
updated_datesource · data ucar educonnector:data_ucar_edu@1.0.0