Data · dataset · 2026
Attribution of Meteorological Variability, Land-Cover/LAI Change, and O<sub>3</sub>‑Induced Stomatal Regulation to Summer Biogenic VOC Emissions in China during 2013–2023
Listed in ZivaHub and Deakin Research Online — shown once because both records carry DOI 10.1021/acs.est.6c08544.s001
Biogenic volatile organic compounds (BVOCs) strongly influence atmospheric oxidation capacity, ozone (O<sub>3</sub>) formation, and secondary organic aerosol production.
Description
In China, BVOC emissions are being reshaped by concurrent meteorological variability, land-cover changes, and increasing surface O<sub>3</sub> pollution, yet their relative contributions remain unclear. Here, we developed an improved WRF-MCIP-BEIS modeling framework incorporating O<sub>3</sub>-induced stomatal regulation through the canopy energy-balance pathway, and integrated O<sub>3</sub>-on/O<sub>3</sub>-off experiments, factorial scenarios, and Shapley decomposition to attribute summer BVOC emission changes across China during 2013–2023.
BVOC emissions exhibited strong regional heterogeneity, with relatively high summer emissions occurring in Southwest China (2019.3 kt summer<sup>–1</sup>), East China (1601.4 kt summer<sup>–1</sup>), and South China (1223.6 kt summer<sup>–1</sup>). O<sub>3</sub>-induced stomatal regulation consistently enhanced summer BVOC emissions, increasing national total emissions by 17.9 kt summer<sup>–1</sup> in 2013 and 29.1 kt summer<sup>–1</sup> in 2023, although the relative effect remained modest (0.20–0.31%).
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Species-level responses were more pronounced: isoprene showed the strongest sensitivity to O<sub>3</sub>-induced stomatal regulation, with relative increases of 0.36–0.55%, approximately two to three times larger than those of other BVOC groups. Shapley decomposition revealed that BVOC emission changes were primarily governed by competing meteorological and land-cover/LAI effects, with national mean contributions of approximately −558.0 and +454.3 kt summer<sup>–1</sup>, respectively, whereas O<sub>3</sub>-induced stomatal regulation accounted for a much smaller but systematic positive scenario-based contribution (+7.6 kt summer<sup>–1</sup>).
These findings demonstrate that O<sub>3</sub>-induced stomatal regulation introduces a modest but chemically relevant vegetation feedback through the canopy energy-balance pathway, while meteorological variability and land-cover/LAI changes remain the dominant controls on long-term summer BVOC variability.
Links
Where it is published
- DOI doi.org/10.1021/acs.est.6c08544.s001 ↗
DOI / persistent id · from zivahub uct ac za
Catalogue records · 1
- OAI-PMH record api.figshare.com/v2/oai?verb=GetRecord&metadataPrefix=oai_dc&identifier=oai%3Af… ↗
metadata API · from zivahub uct ac za
Topics
Related
Provenance · 2 source records, 19 field assertions
| Source | Key | Last seen | Raw |
|---|---|---|---|
| ZivaHub | oai:figshare.com:article/34030263 | 10 d ago | JSON v1 |
| Deakin Research Online | oai:figshare.com:article/34030263 | 10 d ago | JSON v1 |
| Field | Assertion | Extractor | Evidence |
|---|---|---|---|
| access_level | source · zivahub uct ac za | connector:zivahub_uct_ac_za@1.0.0 | |
| concepts[field].anzsrc:group:3103 | mapping · zivahub uct ac za | vocabulary-mapper@1.0.0 | keywords['Ecology'] |
| concepts[field].anzsrc:group:3103 | mapping · dro deakin edu au | vocabulary-mapper@1.0.0 | keywords['Ecology'] |
| concepts[field].anzsrc:group:4410 | mapping · zivahub uct ac za | vocabulary-mapper@1.0.0 | keywords['Sociology'] |
| concepts[field].anzsrc:group:4410 | mapping · dro deakin edu au | vocabulary-mapper@1.0.0 | keywords['Sociology'] |
| concepts[field].local:field:chemistry | mapping · zivahub uct ac za | connector:zivahub_uct_ac_za@1.0.0 | |
| concepts[field].local:field:chemistry | mapping · dro deakin edu au | connector:dro_deakin_edu_au@1.0.0 | |
| concepts[field].local:field:earth-environmental | mapping · zivahub uct ac za | connector:zivahub_uct_ac_za@1.0.0 | |
| concepts[field].local:field:earth-environmental | mapping · dro deakin edu au | connector:dro_deakin_edu_au@1.0.0 | |
| concepts[field].local:field:life-sciences | mapping · zivahub uct ac za | connector:zivahub_uct_ac_za@1.0.0 | |
| concepts[field].local:field:life-sciences | mapping · dro deakin edu au | connector:dro_deakin_edu_au@1.0.0 | |
| concepts[field].local:field:ocean-atmospheric | mapping · zivahub uct ac za | connector:zivahub_uct_ac_za@1.0.0 | |
| concepts[field].local:field:ocean-atmospheric | mapping · dro deakin edu au | connector:dro_deakin_edu_au@1.0.0 | |
| concepts[field].local:field:social-science | mapping · zivahub uct ac za | connector:zivahub_uct_ac_za@1.0.0 | |
| concepts[field].local:field:social-science | mapping · dro deakin edu au | connector:dro_deakin_edu_au@1.0.0 | |
| description | source · zivahub uct ac za | connector:zivahub_uct_ac_za@1.0.0 | /metadata/dc/description |
| license | source · zivahub uct ac za | connector:zivahub_uct_ac_za@1.0.0 | /metadata/dc/rights |
| publication_date | source · zivahub uct ac za | connector:zivahub_uct_ac_za@1.0.0 | |
| title | source · zivahub uct ac za | connector:zivahub_uct_ac_za@1.0.0 | /metadata/dc/title |