Data · dataset · 2022
Vertical distributions of wintertime atmospheric nitrogenous compounds and the corresponding OH radicals production in Leshan, southwest China
Listed in ScienceDB
Ground-based multi-axis differential optical absorption spectroscopy (MAX-DOAS) observations were operated from 02 to 21 December 2018 in Leshan, southwest China, to measure HONO, NO2 and aerosol extinction vertical distributions, and these were the frst MAXDOAS measurement results in Sichuan Basin.
Description
During the measurement period, characteristic ranges for surface concentration were found to be 0.26–4.58 km-1 and averaged at 0.93 km-1 for aerosol extinction, 0.49 to 35.2 ppb and averaged at 4.57 ppb for NO2 and 0.03 to 7.38 ppb and averaged at 1.05 ppb for HONO.
Moreover, vertical profles of aerosol, NO2 and HONO were retrieved from MAX-DOAS measurements using the Heidelberg Profle (HEIPRO) algorithm. By analysing the vertical gradients of pollutants and meteorological information, we found that aerosol and HONO are strongly localised, while NO2 is mainly transmitted from the north direction (city center direction). Nitrogen oxides such as HONO and NO2 are important for the production of hydroxyl radical (OH) and oxidative capacity in the troposphere.
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In this study, the averaged value of OH production rate from HONO is about 0.63 ppb/hr and maximum value of ratio between OH production from HONO and from (HONO+O3) is > 93% before12:00 in Leshan. In addition, combustion emission contributes to 26% for the source of HONO in Leshan, and we found that more NO2 being converted to HONO under the conditions with high aerosol extinction coeffcient and high relative humidity is also a dominant factor for the secondary produce of HONO.
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Where it is published
- DOI doi.org/10.57760/sciencedb.05231 ↗
DOI / persistent id · from scidb cn
Catalogue records · 1
- OAI-PMH record scidb.cn/oai?verb=GetRecord&metadataPrefix=oai_dc&identifier=10.57760%2… ↗
metadata API · from scidb cn
Topics
- From keywords
- Earth & Environmental Science · Engineering · Humanities · Life Sciences · Social Science
Provenance · 1 source records, 9 field assertions
| Source | Key | Last seen | Raw |
|---|---|---|---|
| ScienceDB | 10.57760/sciencedb.05231 | 11 d ago | JSON v1 |
| Field | Assertion | Extractor | Evidence |
|---|---|---|---|
| concepts[field].local:field:earth-environmental | mapping · scidb cn | connector:scidb_cn@1.0.0 | |
| concepts[field].local:field:engineering | mapping · scidb cn | connector:scidb_cn@1.0.0 | |
| concepts[field].local:field:humanities | mapping · scidb cn | connector:scidb_cn@1.0.0 | |
| concepts[field].local:field:life-sciences | mapping · scidb cn | connector:scidb_cn@1.0.0 | |
| concepts[field].local:field:social-science | mapping · scidb cn | connector:scidb_cn@1.0.0 | |
| description | source · scidb cn | connector:scidb_cn@1.0.0 | /metadata/dc/description |
| license_text | source · scidb cn | connector:scidb_cn@1.0.0 | |
| publication_date | source · scidb cn | connector:scidb_cn@1.0.0 | |
| title | source · scidb cn | connector:scidb_cn@1.0.0 | /metadata/dc/title |