Data · dataset · 2026
The effect of support and promoters on the performance of Pt-based H2-SCR catalysts for NOx removal - Raw Data
Listed in RADAR and RADAR4Memory — shown once because both records carry DOI 10.35097/0ne0fakaqd3ay9nh
H₂-combustion engines represent a promising alternative for achieving carbon neutrality.
Description
However, to efficiently remove the resulting NOx emissions, the current H₂-SCR technologies require a more in-depth understanding that will enable further catalyst improvements. In this context, this manuscript reports a systematic study on the effect of support and promoters on the H2-SCR performance of Pt-based catalysts.
Parameters such as catalyst pre-treatment, noble metal loading, space velocity, and gas composition, were varied to elucidate their effects on the measured activity and selectivity profiles and to gain insight into the underlying reaction mechanism. A moderate interaction with the support and the formation of small Pt nanoparticles were identified as essential for NOx conversion at low temperatures. Accordingly, TiO₂-supported catalysts were found to be superior in terms of NOx conversion and N2 yield compared to the CeO₂-supported samples.
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Highly dispersed Pt species as present on strongly interacting supports are also highly sensitive to H2O and O2 inhibition. Acidic promoters increase the activity window, while basic dopants shift and narrow the NOx conversion window toward higher temperatures, the addition of acidic dopants results in the opposite effect. Nevertheless, the presence of basic sites on the catalyst surface improves the N2 selectivity over the operating temperature window and contribute to NH3 formation as secondary
Links
Where it is published
- DOI doi.org/10.35097/0ne0fakaqd3ay9nh ↗
DOI / persistent id · from radar service eu de
Catalogue records · 1
- OAI-PMH record radar-service.eu/oai/OAIHandler?verb=GetRecord&metadataPrefix=oai_dc&identifier… ↗
metadata API · from radar service eu de
Topics
- From keywords
- Earth & Environmental Science · Earth & Environmental Science · Engineering · Engineering
- Inferred from text
- Chemical engineering 71%
Provenance · 2 source records, 10 field assertions
| Source | Key | Last seen | Raw |
|---|---|---|---|
| RADAR | 10.35097/0ne0fakaqd3ay9nh | 11 d ago | JSON v1 |
| RADAR4Memory | 10.35097/0ne0fakaqd3ay9nh | 10 d ago | JSON v1 |
| Field | Assertion | Extractor | Evidence |
|---|---|---|---|
| access_level | source · radar service eu de | connector:radar_service_eu_de@1.0.0 | |
| concepts[field].anzsrc:group:4004 | enrichment · radar service eu de | taxonomy-embedding@1.1.0 | title+keywords+description (71%) |
| concepts[field].local:field:earth-environmental | mapping · radar service eu de | connector:radar_service_eu_de@1.0.0 | |
| concepts[field].local:field:earth-environmental | mapping · radar4memory radar service eu | connector:radar4memory_radar_service_eu@1.0.0 | |
| concepts[field].local:field:engineering | mapping · radar service eu de | connector:radar_service_eu_de@1.0.0 | |
| concepts[field].local:field:engineering | mapping · radar4memory radar service eu | connector:radar4memory_radar_service_eu@1.0.0 | |
| description | source · radar service eu de | connector:radar_service_eu_de@1.0.0 | /metadata/dc/description |
| license | source · radar service eu de | connector:radar_service_eu_de@1.0.0 | /metadata/dc/rights |
| publication_date | source · radar service eu de | connector:radar_service_eu_de@1.0.0 | |
| title | source · radar service eu de | connector:radar_service_eu_de@1.0.0 | /metadata/dc/title |