Replication data for: "Efficient synthesis of well-defined ordered mesoporous aluminosilicates with tailorable acidity"

The publication reports the synthesis and characterization of ordered mesoporous aluminosilicates by direct liquid crystal templating. Take a look at the publication Data files are grouped by measurement method, including (but not limited to): 27Al solid state NMR Total scattering and pair distribution function (PDF) Nitrogen physisorption Pyridine-loaded FTIR spectroscopy (Py-FTIR) Small-angle X-ray scattering (SAXS) Sample names follow the denomination: OMAS_x/1_Tyy — where OMAS = ordered mesoporous aluminosilicate; x/1 = molar Si/Al ratio; Tyy = polycondensation temperature in °C. OMS_Tyy — where OMS = ordered mesoporous silica; Tyy = polycondensation temperature in °C. These datasets support the analysis of how aluminum content and polycondensation temperature influence structural order, pore size, and surface acidity in OMAS.