Constarium
← Search

Data · dataset · 2026

The zonal structure of tropical O₃ and CO as observed by the Tropospheric Emission Spectrometer in November 2004--Part 2: Impact of surface emissions on O₃ and its precursors

Listed in National Center for Atmospheric Research

The impact. of surface emissions on the zonal structure of tropical tropospheric ozone and carbon monoxide is investigated for November 2004 using satellite observations, in-situ measurements, and chemical transport models in conjunction with inverse-estimated surface emissions.

Description

Vertical ozone profiles from the Tropospheric Emission Spectrometer (TES) and ozone sonde measurements from the Southern Hemisphere Additional Ozonesondes (SHADOZ) network show elevated concentrations of ozone over Indonesia and Australia (60-70 ppb) in the lower troposphere against the backdrop of the well-known zonal wave-one pattern with ozone concentrations of (70-80 ppb) centered over the Atlantic.

Observational evidence from TES CO vertical profiles and Ozone Monitoring Instrument (OMI) NO2 columns point to regional surface emissions as an important contributor to the elevated ozone over Indonesia. This contribution is investigated with the GEOS-Chem chemistry and transport model using surface emission estimates derived from an optimal inverse model, which was constrained by TES and Measurements Of Pollution In The Troposphere (MOPITT) CO profiles (Jones et al., 2009).

Read the rest (2 more)

These a posteriori estimates, which were over a factor of 2 greater than climatological emissions, reduced differences between GEOS-Chem and TES ozone observations by 30-40% over Indonesia. The response of the free tropospheric chemical state to the changes in these emissions is investigated for ozone, CO, NOx, and PAN. Model simulations indicate that ozone over Indonesian/Australian is sensitive to regional changes in surface emissions of NOx but relatively insensitive to lightning NOx.

Over sub-equatorial Africa and South America, free tropospheric NOx, was reduced in response to increased surface emissions potentially muting ozone production.

Links

Get the data

Where it is published

Catalogue records · 1

Topics

Inferred from text
Satellite remote sensing 65%
Provenance · 1 source records, 8 field assertions
SourceKeyLast seenRaw
National Center for Atmospheric Researchb8e30254-c097-4316-a01f-02973afbf37610 d agoJSON v1
FieldAssertionExtractorEvidence
concepts[field].local:field:earth-environmentalmapping · data ucar educonnector:data_ucar_edu@1.0.0
concepts[field].local:field:ocean-atmosphericmapping · data ucar educonnector:data_ucar_edu@1.0.0
concepts[modality].local:modality:remote-sensingenrichment · data ucar edukeyword-concept-rules@1.0.0title+description (65%)
created_datesource · data ucar educonnector:data_ucar_edu@1.0.0
descriptionsource · data ucar educonnector:data_ucar_edu@1.0.0/notes
publication_datesource · data ucar educonnector:data_ucar_edu@1.0.0
titlesource · data ucar educonnector:data_ucar_edu@1.0.0/title
updated_datesource · data ucar educonnector:data_ucar_edu@1.0.0