Development and evaluation of E3SM-MOSAIC: Spatial distributions and radiative effects of nitrate aerosol

However, it is not well represented or even neglected in many global climate models. In this study, we couple the Model for Simulating Aerosol Interactions and Chemistry (MOSAIC) module with the four-mode version of the Modal Aerosol Module (MAM4) in DOE's Energy Exascale Earth System Model version 2 (E3SMv2) to simulate nitrate aerosol and its radiative effects.

We find that nitrate aerosol simulated by E3SMv2-MAM4-MOSAIC is sensitive to the treatment of gaseous HNO3 transfer to/from interstitial particles related to accommodation coefficients of HNO3 (urn:x-wiley:19422466:media:jame21740:jame21740-math-0001) on dust and non-dust particles. We compare three different treatments of HNO3 transfer: (a) a treatment (MTC_SLOW) that uses a low urn:x-wiley:19422466:media:jame21740:jame21740-math-0002 in the mass transfer coefficient (MTC) calculation; (b) a dust-weighted MTC treatment (MTC_WGT) that uses a high urn:x-wiley:19422466:media:jame21740:jame21740-math-0003 on non-dust particles; and (c) a dust-weighted MTC treatment that also splits coarse mode aerosols into the coarse dust and sea salt sub-modes in MOSAIC (MTC_SPLC).